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Super-powered lasers to transform nuclear waste

Gerard Mourou
Gérard Mourou
Nobel prize in Physics and member of the Haut Collège de l'École polytechnique

It is no secret that some pro­ducts of nuclear fis­sion are extre­me­ly radio­ac­tive. Trea­ting this waste is the­re­fore one of the big­gest chal­lenges in crea­ting a sus­tai­nable nuclear indus­try. Radio­ac­tive pro­ducts of fis­sion include plu­to­nium (the most com­mon) and other minor acti­nides such as nep­tu­nium, ame­ri­cium and curium, which we find in quan­ti­ties of around 800 grams per ton of spent fuel. Cur­rent­ly, waste pro­ducts from nuclear fis­sion must be secu­re­ly sto­red for extre­me­ly long per­iods of time because of their pro­trac­ted half-lives (the time for their radio­ac­ti­vi­ty to drop by half). Plu­to­nium-239, for example, has a half-life of around 24,000 years.

Along­side secure sto­rage we are now loo­king at how to trans­form, or rather “trans­mute”, this waste with the help of power­ful lasers so that it can be bet­ter mana­ged. Theo­re­ti­cal­ly, these lasers are power­ful enough to sti­mu­late nuclear fis­sion in plu­to­nium and other minor acti­nides (cur­rent­ly the most hazar­dous waste). In short, trans­mu­ta­tion treats waste from nuclear fis­sion in two ways. Either by conver­ting it into sub-pro­ducts with wea­ker ato­mic masses and much shor­ter half-lives. Or by adding par­ticles to create less radio­ac­tive iso­topes, which also shor­tens very long half-lives – some­times down to just one year.

We are loo­king at how to trans­form, or rather “trans­mute”, nuclear waste with the help of power­ful lasers.

Amplified laser power

We hope to be able to achieve trans­mu­ta­tion of nuclear waste using chir­ped pulse ampli­fi­ca­tion (CPA). With this tech­nique, the extreme light from lasers can be boos­ted to levels long thought impos­sible, mea­su­red in peta­watts (PW) – the equi­va­lent of 1015 watts. To give an idea of scale, one PW is around fif­ty times the power of the world’s entire elec­tric grid, and the total ener­gy the earth receives from the sun is mea­su­red at 174 PW.

CPA uses an ultra-short laser pulse, sprea­ding out its spec­tral com­po­nents before ampli­fi­ca­tion. The pulse is then com­pres­sed again for a very short time, gene­ra­ting enough power to create par­ticles (elec­trons and pro­tons) by deta­ching them from mat­ter, before acce­le­ra­ting these par­ticles using conven­tio­nal tech­niques. These kinds of lasers are alrea­dy ope­ra­tio­nal – no small feat since one of the chal­lenges was to create a mecha­nism that would not be des­troyed by the power of the beam itself ! And we also know how to detach par­ticles. Howe­ver, the chal­lenge is now around effi­cien­cy : how do we make these lasers small enough and at suf­fi­cient scales without consu­ming too much ener­gy in the pro­cess ? It is the­re­fore a pro­blem around indus­trial pro­duc­tion – a pro­blem that the XCAN pro­ject is spe­ci­fi­cal­ly desi­gned to meet.

An alternative to uranium

On top of that, a CPA-boos­ted laser could be used to gene­rate fis­sion, pro­vi­ding an alter­na­tive to the neu­tron bom­bard­ment method used in cur­rent reac­tors. This is an option we are explo­ring, and which could be pivo­tal for deve­lo­ping tho­rium-based power. Tho­rium is a hea­vy metal found in far grea­ter quan­ti­ties around the world than ura­nium ; in theo­ry, it could pro­vide a repla­ce­ment for ura­nium in nuclear power. Moreo­ver, the by-pro­ducts of tho­rium fis­sion are also less hazar­dous than ura­nium and have shor­ter half-lives of just a few hun­dred years. Given that this kind of fis­sion does not pro­duce plu­to­nium, it is also a good option for pure­ly civil nuclear appli­ca­tions, without the risks sur­roun­ding pro­duc­tion of nuclear weapons.

But tho­rium fis­sion is dif­fi­cult, invol­ving an extra step as com­pa­red to ura­nium fis­sion. The tho­rium must first be brought to a sub­cri­ti­cal level ; neu­trons from an exter­nal source are then used to pro­voke fis­sion. Lasers could play a key role in this pro­cess prior to fis­sion, in par­ti­cu­lar because they allow for a high level of control. The sys­tem can be fed with a constant light source, simi­lar to ope­ra­ting a tap.

Many phy­si­cists, inclu­ding myself, are convin­ced of the poten­tial of tho­rium-based power. But while it is scien­ti­fi­cal­ly sound, there are still many tech­ni­cal pro­blems to be sol­ved. In par­ti­cu­lar, concer­ning the ener­gy requi­red to gene­rate fis­sion. But lasers could be part of the solution.

Contributors

Gerard Mourou

Gérard Mourou

Nobel prize in Physics and member of the Haut Collège de l'École polytechnique

Gérard Mourou has spent a large part of his career in the United States, in particular at the University of Michigan, where he is now Professor Emeritus. Upon his return to France in 2005, he was head of the Applied optics laboratory (a UMR ENSTA ParisTech/CNRS/École polytechnique) until 2008. Gérard Mourou is a Knight of the legion of honour. His awards include the Frederic Ives medal (2016) from the Optical society of America and the Arthur L. Schawlow prize in laser science from the American Physical Society in 2018. Gérard Mourou received the Nobel Prize in Physics in 2018, which crowns a career dedicated entirely to lasers and physics.

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