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Super-powered lasers to transform nuclear waste

Gerard Mourou
Gérard Mourou
Nobel prize in Physics and member of the Haut Collège de l'École polytechnique

It is no secret that some products of nuc­le­ar fis­sion are extremely radio­act­ive. Treat­ing this waste is there­fore one of the biggest chal­lenges in cre­at­ing a sus­tain­able nuc­le­ar industry. Radio­act­ive products of fis­sion include plutoni­um (the most com­mon) and oth­er minor actin­ides such as nep­tuni­um, amer­i­ci­um and curi­um, which we find in quant­it­ies of around 800 grams per ton of spent fuel. Cur­rently, waste products from nuc­le­ar fis­sion must be securely stored for extremely long peri­ods of time because of their pro­trac­ted half-lives (the time for their radio­activ­ity to drop by half). Plutoni­um-239, for example, has a half-life of around 24,000 years.

Along­side secure stor­age we are now look­ing at how to trans­form, or rather “trans­mute”, this waste with the help of power­ful lasers so that it can be bet­ter man­aged. The­or­et­ic­ally, these lasers are power­ful enough to stim­u­late nuc­le­ar fis­sion in plutoni­um and oth­er minor actin­ides (cur­rently the most haz­ard­ous waste). In short, trans­mu­ta­tion treats waste from nuc­le­ar fis­sion in two ways. Either by con­vert­ing it into sub-products with weak­er atom­ic masses and much short­er half-lives. Or by adding particles to cre­ate less radio­act­ive iso­topes, which also shortens very long half-lives – some­times down to just one year.

We are look­ing at how to trans­form, or rather “trans­mute”, nuc­le­ar waste with the help of power­ful lasers.

Amplified laser power

We hope to be able to achieve trans­mu­ta­tion of nuc­le­ar waste using chirped pulse amp­li­fic­a­tion (CPA). With this tech­nique, the extreme light from lasers can be boos­ted to levels long thought impossible, meas­ured in pet­awatts (PW) – the equi­val­ent of 1015 watts. To give an idea of scale, one PW is around fifty times the power of the world’s entire elec­tric grid, and the total energy the earth receives from the sun is meas­ured at 174 PW.

CPA uses an ultra-short laser pulse, spread­ing out its spec­tral com­pon­ents before amp­li­fic­a­tion. The pulse is then com­pressed again for a very short time, gen­er­at­ing enough power to cre­ate particles (elec­trons and pro­tons) by detach­ing them from mat­ter, before accel­er­at­ing these particles using con­ven­tion­al tech­niques. These kinds of lasers are already oper­a­tion­al – no small feat since one of the chal­lenges was to cre­ate a mech­an­ism that would not be des­troyed by the power of the beam itself! And we also know how to detach particles. How­ever, the chal­lenge is now around effi­ciency: how do we make these lasers small enough and at suf­fi­cient scales without con­sum­ing too much energy in the pro­cess? It is there­fore a prob­lem around indus­tri­al pro­duc­tion – a prob­lem that the XCAN pro­ject is spe­cific­ally designed to meet.

An alternative to uranium

On top of that, a CPA-boos­ted laser could be used to gen­er­ate fis­sion, provid­ing an altern­at­ive to the neut­ron bom­bard­ment meth­od used in cur­rent react­ors. This is an option we are explor­ing, and which could be pivotal for devel­op­ing thori­um-based power. Thori­um is a heavy met­al found in far great­er quant­it­ies around the world than urani­um; in the­ory, it could provide a replace­ment for urani­um in nuc­le­ar power. Moreover, the by-products of thori­um fis­sion are also less haz­ard­ous than urani­um and have short­er half-lives of just a few hun­dred years. Giv­en that this kind of fis­sion does not pro­duce plutoni­um, it is also a good option for purely civil nuc­le­ar applic­a­tions, without the risks sur­round­ing pro­duc­tion of nuc­le­ar weapons.

But thori­um fis­sion is dif­fi­cult, involving an extra step as com­pared to urani­um fis­sion. The thori­um must first be brought to a sub­crit­ic­al level; neut­rons from an extern­al source are then used to pro­voke fis­sion. Lasers could play a key role in this pro­cess pri­or to fis­sion, in par­tic­u­lar because they allow for a high level of con­trol. The sys­tem can be fed with a con­stant light source, sim­il­ar to oper­at­ing a tap.

Many phys­i­cists, includ­ing myself, are con­vinced of the poten­tial of thori­um-based power. But while it is sci­en­tific­ally sound, there are still many tech­nic­al prob­lems to be solved. In par­tic­u­lar, con­cern­ing the energy required to gen­er­ate fis­sion. But lasers could be part of the solution.

Contributors

Gerard Mourou

Gérard Mourou

Nobel prize in Physics and member of the Haut Collège de l'École polytechnique

Gérard Mourou has spent a large part of his career in the United States, in particular at the University of Michigan, where he is now Professor Emeritus. Upon his return to France in 2005, he was head of the Applied optics laboratory (a UMR ENSTA ParisTech/CNRS/École polytechnique) until 2008. Gérard Mourou is a Knight of the legion of honour. His awards include the Frederic Ives medal (2016) from the Optical society of America and the Arthur L. Schawlow prize in laser science from the American Physical Society in 2018. Gérard Mourou received the Nobel Prize in Physics in 2018, which crowns a career dedicated entirely to lasers and physics.

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